Malmö University Publications
Planned maintenance
A system upgrade is planned for 10/12-2024, at 12:00-13:00. During this time DiVA will be unavailable.
Change search
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf
Hydration-Induced Structural Changes in the Solid State of Protein: A SAXS/WAXS Study on Lysozyme.
Malmö University, Faculty of Health and Society (HS), Department of Biomedical Science (BMV). Malmö University, Biofilms Research Center for Biointerfaces. Max IV Laboratory, Lund University, 224 84 Lund, Sweden.ORCID iD: 0000-0003-1091-1468
Malmö University, Faculty of Health and Society (HS), Department of Biomedical Science (BMV). Malmö University, Biofilms Research Center for Biointerfaces.ORCID iD: 0000-0003-2233-1436
RISE Research Institutes of Sweden, 114 86 Stockholm, Sweden.
SOBI Swedish Orphan Biovitrum, 112 76 Stockholm, Sweden.
Show others and affiliations
2020 (English)In: Molecular Pharmaceutics, ISSN 1543-8384, E-ISSN 1543-8392, Vol. 17, no 9, p. 3246-3258Article in journal (Refereed) Published
Abstract [en]

The stability of biologically produced pharmaceuticals is the limiting factor to various applications, which can be improved by formulation in solid-state forms, mostly via lyophilization. Knowledge about the protein structure at the molecular level in the solid state and its transition upon rehydration is however scarce, and yet it most likely affects the physical and chemical stability of the biological drug. In this work, synchrotron small- and wide-angle X-ray scattering (SWAXS) are used to characterize the structure of a model protein, lysozyme, in the solid state and its structural transition upon rehydration to the liquid state. The results show that the protein undergoes distortion upon drying to adopt structures that can continuously fill the space to remove the protein-air interface that may be formed upon dehydration. Above a hydration threshold of 35 wt %, the native structure of the protein is recovered. The evolution of SWAXS peaks as a function of water content in a broad range of concentrations is discussed in relation to the structural changes in the protein. The findings presented here can be used for the design and optimization of solid-state formulations of proteins with improved stability.

Place, publisher, year, edition, pages
American Chemical Society (ACS), 2020. Vol. 17, no 9, p. 3246-3258
Keywords [en]
biotherapeutics, dehydration, distorted structure, hydration, small- and wide-angle X-ray scattering, solid-state protein
National Category
Biochemistry and Molecular Biology
Identifiers
URN: urn:nbn:se:mau:diva-18376DOI: 10.1021/acs.molpharmaceut.0c00351ISI: 000571389900009PubMedID: 32787275Scopus ID: 2-s2.0-85090505313OAI: oai:DiVA.org:mau-18376DiVA, id: diva2:1469917
Available from: 2020-09-23 Created: 2020-09-23 Last updated: 2024-06-17Bibliographically approved

Open Access in DiVA

fulltext(2132 kB)277 downloads
File information
File name FULLTEXT01.pdfFile size 2132 kBChecksum SHA-512
37e72a545f94f9ba63970275dec2591326fe9ab805b9aec451dc2ff4e2b3100fe56e78f70c03b94d6911046153cec5436d43a63dee577136b3c6084078fa3111
Type fulltextMimetype application/pdf

Other links

Publisher's full textPubMedScopus

Authority records

Phan-Xuan, TuanBogdanova, EkaterinaKocherbitov, Vitaly

Search in DiVA

By author/editor
Phan-Xuan, TuanBogdanova, EkaterinaKocherbitov, Vitaly
By organisation
Department of Biomedical Science (BMV)Biofilms Research Center for Biointerfaces
In the same journal
Molecular Pharmaceutics
Biochemistry and Molecular Biology

Search outside of DiVA

GoogleGoogle Scholar
Total: 277 downloads
The number of downloads is the sum of all downloads of full texts. It may include eg previous versions that are now no longer available

doi
pubmed
urn-nbn

Altmetric score

doi
pubmed
urn-nbn
Total: 172 hits
CiteExportLink to record
Permanent link

Direct link
Cite
Citation style
  • apa
  • ieee
  • modern-language-association-8th-edition
  • vancouver
  • Other style
More styles
Language
  • de-DE
  • en-GB
  • en-US
  • fi-FI
  • nn-NO
  • nn-NB
  • sv-SE
  • Other locale
More languages
Output format
  • html
  • text
  • asciidoc
  • rtf